成碧君, 杨秀娟, 高林英, 刘良坡, 张红梅. 山西省某煤矿区土壤重金属类金属污染与健康风险评估[J]. 环境卫生学杂志, 2022, 12(5): 332-344. DOI: 10.13421/j.cnki.hjwsxzz.2022.05.003
    引用本文: 成碧君, 杨秀娟, 高林英, 刘良坡, 张红梅. 山西省某煤矿区土壤重金属类金属污染与健康风险评估[J]. 环境卫生学杂志, 2022, 12(5): 332-344. DOI: 10.13421/j.cnki.hjwsxzz.2022.05.003
    CHENG Bi-jun, YANG Xiu-juan, GAO Lin-ying, LIU Liang-po, ZHANG Hong-mei. Metal and metalloid pollution and health risk assessment in a coal mine area of Shanxi Province, China[J]. Journal of Environmental Hygiene, 2022, 12(5): 332-344. DOI: 10.13421/j.cnki.hjwsxzz.2022.05.003
    Citation: CHENG Bi-jun, YANG Xiu-juan, GAO Lin-ying, LIU Liang-po, ZHANG Hong-mei. Metal and metalloid pollution and health risk assessment in a coal mine area of Shanxi Province, China[J]. Journal of Environmental Hygiene, 2022, 12(5): 332-344. DOI: 10.13421/j.cnki.hjwsxzz.2022.05.003

    山西省某煤矿区土壤重金属类金属污染与健康风险评估

    Metal and metalloid pollution and health risk assessment in a coal mine area of Shanxi Province, China

    • 摘要:
      目的 了解山西煤矿区农田土壤重金属/类金属污染的来源、污染特征及其健康风险。
      方法 研究测定了山西省某煤矿区农田土壤样本中重金属/类金属含量, 分析矿区土壤重金属/类金属污染特征, 基于主成分/绝对主成分受体模型(principal component analysis/absolute principal component score receptor model, PCA/APCS)开展污染来源分析, 通过健康风险评价评估周围居民的健康风险。
      结果 结果表明该煤矿污染区: ①Zn、Cu、Cr和As的浓度均显著高于对照区, As浓度是风险管制值的(3.4~4.3)倍; ②研究区域内梅罗指数为4.34, 表示土壤处于重金属/类金属复合重度污染; 污染负荷指数为1.59, 土壤污染负荷处于轻度水平; 综合潜在生态风险指数为32.89, 土壤生态处于轻度风险; ③源解析结果显示土壤重金属Zn、Ni和Cu受煤矿开采、煤炭运输和农业活动等人类活动影响, As和Cr主要来自自然活动影响; ④非致癌风险指数均未超过1, 重金属/类金属污染对人体健康产生的非致癌风险甚微; Ni、Cr和As的致癌风险指数处于10-6~10-4之间, 表明这些重金属/类金属对人体健康存在一定的致癌风险, 但尚在可接受范围内。
      结论 煤矿污染区土壤重金属/类金属分布存在明显差异, 其重金属/类金属复合污染有必要引起重视; 尽管研究区域的土壤重金属/类金属污染引起的健康风险均未超过阈值, 但土壤污染防治丝毫不容怠懈, 对土壤重金属/类金属健康风险应提高警惕, 加强预警。

       

      Abstract:
      Objective To investigate the pollution characteristics, pollution sources, and health risks of metal and metalloid in farmland soil in coal mine areas of Shanxi Province, China.
      Methods The contents of metal and metalloid were determined for the farmland soil samples from a coal mine area of Shanxi province, and the characteristics of metal and metalloid pollution were analyzed in soil samples. The principal component analysis/absolute principal component score receptor model (PCA/APCS) was used to investigate pollution sources, and the health risk assessment index system was used to analyze the health risks of residents around the mine area.
      Results The result showed that the mass concentrations of Zn, Cu, Cr, and As in the polluted area were significantly higher than those in the control area, and the mass concentration of As was 3.4-4.3 times of the risk control value for metalloids. The study area had a Nemerow index of 4.34, which showed the presence of severe combined pollution of metal and metalloid in soil. The pollution load index was 1.59, indicating a mild level of metal and metalloid pollution load in soil. The potential ecological risk index of the study area was 32.89, suggesting a mild risk of soil ecology. Source apportionment showed that the heavy metals of Zn, Ni, and Cu in soil were affected by human activities such as coal mining, coal transportation and agricultural activities, and As and Cr were mainly affected by nature activities. The non-carcinogenic risk index did not exceed the threshold value of 1, indicating that metal and metalloid pollution posed little non-carcinogenic risk to human health. The carcinogenic risk index of Ni, Cr, and As ranged from 10-6 to 10-4, indicating that these metal and metalloid posed a certain carcinogenic risk to human health, which was within an acceptable range.
      Conclusion There is a significant difference in the distribution of metal and metalloid in soil of polluted coal mine area, and combined metal and metalloid pollution should be taken seriously. Although the health risk caused by soil metal and metalloid pollution does not exceed the threshold, the prevention and control of soil pollution should be performed actively. The health risk of soil metal and metalloid should be closely monitored to strengthen early warning.

       

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